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Thesis

Activation of small molecules by solid-supported frustrated Lewis pairs

Abstract:

The aims of this thesis have been to develop heterogeneous frustrated Lewis pairs for the catalytic activation of small molecules. Frustrated Lewis pairs capable of H2 activation and CO2 hydrogenation based on electron-deficient tri-aryl boranes and sterically encumbered phosphines have been immobilised on silica. The reactivity of these heterogeneous systems with small molecules has been tested and compared with a variety of soluble siloxane and silsesquioxane molecu...

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Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author

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Role:
Supervisor
Type of award:
DPhil
Level of award:
Doctoral
Awarding institution:
University of Oxford
UUID:
uuid:cb32a5a7-8613-413f-b47c-80674e904c3a
Deposit date:
2017-06-18

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