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Revealing the origin of voltage loss in mixed-halide perovskite solar cells

Abstract:

The tunable bandgap of metal-halide perovskites has opened up the possibility of tandem solar cells with over 30% efficiency. Iodide-Bromide (I-Br) mixed-halide perovskites are crucial to achieve the optimum bandgap for such tandems. However, when the Br content is increased to widen the bandgap, cells fail to deliver the expected increase in open-circuit voltage (VOC). This loss in VOC has been attributed to photo-induced halide segregation. Here, we combine Fourier Transform Photocurrent Sp...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1039/c9ee02162k

Authors


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Institution:
University of Oxford
Department:
Physics
Sub department:
Condensed Matter Physics
Oxford college:
Worcester College
Role:
Author
Publisher:
Royal Society of Chemistry
Journal:
Energy and Environmental Science More from this journal
Volume:
13
Pages:
258-267
Publication date:
2019-11-26
Acceptance date:
2019-11-26
DOI:
EISSN:
1754-5706
ISSN:
1754-5692
Language:
English
Keywords:
Pubs id:
pubs:1074726
UUID:
uuid:67b313e3-e802-44b9-9d6f-e462c08d2d4e
Local pid:
pubs:1074726
Source identifiers:
1074726
Deposit date:
2019-11-28

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