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Probing the molecular basis of photochemistry and photophysics with vibrational coherence spectroscopy

Abstract:

We present a time-domain impulsive vibrational spectroscopy (IVS) setup capable of recording background- and baseline-free Raman spectra of excited electronic states in condensed-phase molecular systems. The setup records vibrational Raman spectra from 50-3000 cm-1 and is readily extended to follow spectral evolutions with a time resolution of <20 fs, opening up the possibility for multi-dimensional Raman spectroscopy. Based on the setup, we explore a wide range of photoc...

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Division:
MPLS
Department:
Chemistry
Role:
Author

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Role:
Supervisor
Type of award:
DPhil
Level of award:
Doctoral
Awarding institution:
University of Oxford
Language:
English
Subjects:
UUID:
uuid:0fbfdfe7-13e6-4118-bfc0-2bff5f61834a
Deposit date:
2016-01-22

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