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Rhodium catalysed hydroacylation reactions in the synthesis of heterocycles

Abstract:

Rhodium-catalysed hydroacylation provides a highly atom economic synthesis of ketone products from the combination of aldehydes and multiple bond systems by C-H bond activation. This work evaluates the combination of intermolecular hydroacylation for the synthesis of classical heterocycle precursors and their dehydrative cyclisation to give rise to a range of substituted heterocyclic compounds.

Chapter 1 outlines recent developments in the chemistry of hydroacylation. Particular atte...

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Institution:
University of Oxford
Research group:
Willis Group
Oxford college:
Brasenose College
Department:
Mathematical,Physical & Life Sciences Division - Chemistry - Organic Chemistry
Role:
Author

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Supervisor
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Funding agency for:
Paul M. Ylioja
Publication date:
2011
Type of award:
DPhil
Level of award:
Doctoral
Awarding institution:
Oxford University, UK
URN:
uuid:0bd31ddc-c13e-4502-b359-64495a297489
Local pid:
ora:5671

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