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Handle on the antiferromagnetic spin structure of NiO using a ferromagnetic adlayer

Abstract:
Antiferromagnets (AFs) are characterized by spin structures that are resistant to external magnetic fields, rendering them ideal for persistent information storage but challenging to control. This study demonstrates that a thin ferromagnetic adlayer can serve as a magnetic ‘lever’ to provide a strong handle on the spin texture of an adjacent antiferromagnet. In bilayers composed of NiO(001) and Co, the expected exchange bias effect—a unidirectional shift in the Co hysteresis due to coupling with NiO—is notably absent. Instead, a strong interfacial coupling is observed, causing the NiO to partially follow the magnetization of Co under an applied magnetic field. Using x-ray magnetic linear dichroism, we detect an inversion of dichroism, indicating a reorientation of the Néel vector in NiO. X-ray spectromicroscopy imaging further reveals a direct correlation between ferromagnetic and antiferromagnetic domain structures. These findings are explained using a toy model that distinguishes between stable and unstable AF domains, highlighting the dynamic interplay between NiO and the Co adlayer in the presence of a magnetic field.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/physrevmaterials.9.014408

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Role:
Author
ORCID:
0000-0002-3977-4623
More by this author
Role:
Author
ORCID:
0000-0001-6852-2495


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Funder identifier:
https://ror.org/0439y7842
Grant:
2604894


Publisher:
American Physical Society
Journal:
Physical Review Materials More from this journal
Volume:
9
Issue:
1
Article number:
014408
Publication date:
2025-01-27
Acceptance date:
2025-01-10
DOI:
EISSN:
2475-9953


Language:
English
Pubs id:
2080975
Local pid:
pubs:2080975
Deposit date:
2025-01-28

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