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Efficient dynamic nuclear polarization at high magnetic fields

Abstract:
By applying a new technique for dynamic nuclear polarization involving simultaneous excitation of electronic and nuclear transitions, we have enhanced the nuclear polarization of the nitrogen nuclei in N15@C60 by a factor of 103 at a fixed temperature of 3 K and a magnetic field of 8.6 T, more than twice the maximum enhancement reported to date. This methodology will allow the initialization of the nuclear qubit in schemes exploiting N@C60 molecules as components of a quantum information processing device. © 2007 The American Physical Society.

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Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
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Institution:
University of Oxford
Division:
MPLS
Department:
Materials
Role:
Author
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Journal:
Physical Review Letters
Volume:
98
Issue:
22
Publication date:
2007-05-31
DOI:
EISSN:
1079-7114
ISSN:
0031-9007
Source identifiers:
178556
Language:
English
Pubs id:
pubs:178556
UUID:
uuid:f9ebce22-06f1-4071-b45b-f51d904aab6e
Local pid:
pubs:178556
Deposit date:
2012-12-19

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