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Hydrogen-bonded homoleptic fluoride–diarylurea complexes: structure, reactivity, and coordinating power

Abstract:

Hydrogen bonding with fluoride is a key interaction encountered when analyzing the mode of action of 5′-fluoro-5′-deoxyadenosine synthase, the only known enzyme capable of catalyzing the formation of a C–F bond from F–. Further understanding of the effect of hydrogen bonding on the structure and reactivity of complexed fluoride is therefore important for catalysis and numerous other applications, such as anion supramolecular chemistry. Herein we disclose a detailed study examining the structu...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/jacs.6b07501

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Role:
Author
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National Science Foundation More from this funder
Scripps Research Institute More from this funder
University Of Oxford More from this funder
Wolfson Foundation More from this funder
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Grant:
FP7-PEOPLE-2012-ITN-RADIOMI-316882
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Publisher:
American Chemical Society Publisher's website
Journal:
Journal of the American Chemical Society Journal website
Volume:
138
Issue:
40
Pages:
13314-13325
Publication date:
2016-09-08
Acceptance date:
2016-09-08
DOI:
EISSN:
1520-5126
ISSN:
0002-7863
Pmid:
27608274
Pubs id:
pubs:648050
UUID:
uuid:f810cea0-2806-4be9-b735-9fe34762d31f
Source identifiers:
648050
Local pid:
pubs:648050
Language:
English

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