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Palladium-catalyzed cyclization of bromoenynamides to tricyclic azacycles: synthesis of trikentrin-like frameworks.

Abstract:
Palladium-catalyzed cascade cyclization of bromoenynamides equipped with an additional alkyne or ynamide substituent affords azatricyclic products. Using 5- to 7-membered ring tethers, this chemistry offers a regiospecific route to highly-functionalized azacycles. Elaboration to the trikentrin B skeleton is achieved from the arylsilane cyclization products.
Publication status:
Published

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Publisher copy:
10.1039/c3cc45634j

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Organic Chemistry
Role:
Author
Journal:
Chemical Communications More from this journal
Volume:
50
Issue:
40
Pages:
5187-5189
Publication date:
2014-05-01
DOI:
EISSN:
1364-548X
ISSN:
1359-7345
Language:
English
Keywords:
Pubs id:
pubs:420916
UUID:
uuid:f6c5411b-ecc9-4b08-8cd3-48688e947f86
Local pid:
pubs:420916
Source identifiers:
420916
Deposit date:
2013-11-17

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