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Hard carbon from a sugar derivative for next-generation sodium-ion batteries

Abstract:
Sodium-ion batteries have emerged as a promising secondary battery system due to the abundance of sodium resources. One of the boosters for accelerating the practical application of sodium-ion batteries is the innovation in anode materials. This study focuses on developing a high-performance hard carbon anode material derived from hydroxymethylfurfural, produced from carbohydrates, using a straightforward thermal condensation method. The process results in a unique pseudo-graphitic material with abundant microporosity. Electrochemical evaluations demonstrate excellent sodium storage performance by maintaining the plateau capacity even at higher current densities. This translates to a promising energy density when coupled with the cathode material. However, we also discuss the influence of electrolyte composition on the performance of the hydroxymethylfurfural-derived hard carbon, emphasizing the critical role of electrolyte optimization for the development of efficient and sustainable carbonaceous anode materials for next-generation sodium-based batteries.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1039/d4mh01118j

Authors

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Role:
Author
ORCID:
0000-0002-5364-6791
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Institution:
University of Oxford
Division:
MPLS
Department:
Engineering Science
Role:
Author
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Role:
Author
ORCID:
0000-0003-3314-6906


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Funder identifier:
https://ror.org/0472cxd90
Grant:
951513


Publisher:
Royal Society of Chemistry
Journal:
Materials Horizons More from this journal
Volume:
12
Issue:
3
Pages:
886-898
Place of publication:
England
Publication date:
2025-02-03
Acceptance date:
2024-10-24
DOI:
EISSN:
2051-6355
ISSN:
2051-6347
Pmid:
39535409


Language:
English
Pubs id:
2062888
Local pid:
pubs:2062888
Deposit date:
2025-02-26
ARK identifier:

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