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Dependence of the nascent vibrational distribution of NO(v) on the photolysis wavelength of NO2 in the range lambda = 266-327 nm measured by time-resolved Fourier transform infrared emission.

Abstract:

Time-resolved FTIR has been used to study the photodissociation of NO2 at photolysis wavelengths of lambda = 266, 282, 295, 308, 320 and 327 nm. Nascent vibrational distributions of the NO(v) fragment have been determined at all wavelengths: 266 nm photolysis populates NO(v = 1-7) and shows a distribution that is inverted at v = 5, whereas 327 nm photolysis populates NO(v = 1-3) and is inverted at v = 2. Surprisal plots were performed on the nascent distributions presented in this work and on...

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Publication status:
Published

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Publisher copy:
10.1039/b710594k

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
Journal:
Physical chemistry chemical physics : PCCP More from this journal
Volume:
9
Issue:
38
Pages:
5232-5240
Publication date:
2007-10-01
DOI:
EISSN:
1463-9084
ISSN:
1463-9076
Language:
English
Pubs id:
pubs:34731
UUID:
uuid:e951d172-ea1f-466f-97e8-170fbd7294b2
Local pid:
pubs:34731
Source identifiers:
34731
Deposit date:
2012-12-19

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