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Magnetic monopole density and antiferromagnetic domain control in spin-ice iridates

Abstract:
Magnetically frustrated systems provide fertile ground for complex behaviour, including unconventional ground states with emergent symmetries, topological properties, and exotic excitations. A canonical example is the emergence of magnetic-charge-carrying quasiparticles in spin-ice compounds. Despite extensive work, a reliable experimental indicator of the density of these magnetic monopoles is yet to be found. Using measurements on single crystals of Ho2Ir2O7 combined with dipolar Monte Carlo simulations, we show that the isothermal magnetoresistance is highly sensitive to the monopole density. Moreover, we uncover an unexpected and strong coupling between the monopoles on the holmium sublattice and the antiferromagnetically ordered iridium ions. These results pave the way towards a quantitative experimental measure of monopole density and demonstrate the ability to control antiferromagnetic domain walls using a uniform external magnetic field, a key goal in the design of next-generation spintronic devices.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1038/s41467-022-27964-y

Authors


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Role:
Author
ORCID:
0000-0001-9108-9490
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Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Role:
Author
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Role:
Author
ORCID:
0000-0002-2270-2295


Publisher:
Springer Nature
Journal:
Nature Communications More from this journal
Volume:
13
Issue:
1
Article number:
444
Publication date:
2022-01-21
Acceptance date:
2021-12-22
DOI:
EISSN:
2041-1723
Pmid:
35064100


Language:
English
Keywords:
Pubs id:
1235864
Local pid:
pubs:1235864
Deposit date:
2022-03-21

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