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All-in all-out magnetic order and propagating spin-waves in Sm2Ir2O7

Abstract:
Using resonant magnetic x-ray scattering we address the unresolved nature of the magnetic groundstate and the low-energy effective Hamiltonian of Sm2Ir2O7, a prototypical pyrochlore iridate with a finite temperature metal-insulator transition. Through a combination of elastic and inelastic measurements, we show that the magnetic ground state is an all-in all-out (AIAO) antiferromagnet. The magnon dispersion indicates significant electronic correlations and can be well-described by a minimal Hamiltonian that includes Heisenberg exchange (J = 27.3(6) meV) and DzyaloshinskiiMoriya interaction (D = 4.9(3) meV), which provides a consistent description of the magnetic order and excitations. In establishing that Sm2Ir2O7 has the requisite inversion symmetry preserving AIAO magnetic groundstate, our results support the notion that pyrochlore iridates may host correlated Weyl semimetals.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/PhysRevLett.117.037201

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author


Publisher:
American Physical Society
Journal:
Physical Review Letters More from this journal
Volume:
117
Issue:
3
Pages:
037201
Publication date:
2016-07-11
Acceptance date:
2016-05-25
DOI:
EISSN:
1079-7114
ISSN:
0031-9007


Pubs id:
pubs:632209
UUID:
uuid:c8d55b03-059e-42a1-9673-3a995d525ed6
Local pid:
pubs:632209
Source identifiers:
632209
Deposit date:
2016-07-06

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