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Groups 1, 2 and Zn(II) heterodinuclear catalysts for epoxide/CO2 ring-opening copolymerization

Abstract:

A series of heterodinuclear complexes are reported where both Zn(II) and a metal from Group 1 or 2 are chelated by a macrocyclic diphenolate-tetra-amine ligand. The complexes are characterized in the solid state, where relevant by single crystal X-ray crystallography and elemental analysis, and in solution, using NMR spectroscopy and mass spectrometry. The complex synthesis is achieved by reaction of the ligand with diethyl zinc to form the monozinc complex, in situ, followed by subsequent co...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/acs.inorgchem.8b02923

Authors


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Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
More by this author
Role:
Author
ORCID:
0000-0001-7569-6856
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Oxford college:
Trinity College
Role:
Author
ORCID:
0000-0002-0734-1575
Publisher:
American Chemical Society Publisher's website
Journal:
Inorganic Chemistry Journal website
Volume:
57
Issue:
24
Pages:
15575-15583
Publication date:
2018-11-30
Acceptance date:
2018-11-14
DOI:
EISSN:
1520-510X
ISSN:
0020-1669
Pmid:
30499670
Language:
English
Pubs id:
pubs:952213
UUID:
uuid:c748effc-a838-48f1-b84d-e557e63ac5df
Local pid:
pubs:952213
Source identifiers:
952213
Deposit date:
2019-02-08

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