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Spin dynamics of coupled spin ladders near quantum criticality in Ba2CuTeO6

Abstract:
We report inelastic neutron scattering measurements of the magnetic excitations in Ba2CuTeO6, proposed by ab initio calculations to magnetically realize weakly coupled antiferromagnetic two-leg spin-1/2 ladders. Isolated ladders are expected to have a singlet ground state protected by a spin gap. Ba2CuTeO6 orders magnetically, but with a small Neel temperature relative to the exchange strength, suggesting that the interladder couplings are relatively small and only just able to stabilize magnetic order, placing Ba2CuTeO6 close in parameter space to the critical point separating the gapped phase and Neel order. Through comparison of the observed spin dynamics with linear spin wave theory and quantum Monte Carlo calculations, we propose values for all relevant intra- and interladder exchange parameters, which place the system on the ordered side of the phase diagram in proximity to the critical point. We provide further cross-checks of the extracted parameters by comparison with high field magnetization data.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/PhysRevB.98.174410

Authors


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Institution:
University of Oxford
Division:
MPLS Division
Department:
Physics
Sub department:
Condensed Matter Physics
Oxford college:
Mansfield College
Role:
Author


More from this funder
Funding agency for:
Macdougal, D
Grant:
Doctoral studentship
EP/M020517/1


Publisher:
American Physical Society
Journal:
Physical review B: Condensed matter and materials physics More from this journal
Volume:
98
Pages:
174410
Publication date:
2018-11-07
Acceptance date:
2018-10-03
DOI:
EISSN:
1550-235X
ISSN:
1098-0121


Pubs id:
pubs:858738
UUID:
uuid:c2e8821f-0f69-40f5-8e29-86c81367d8c3
Local pid:
pubs:858738
Source identifiers:
858738
Deposit date:
2018-10-08

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