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Synthesis of five-porphyrin nanorings by using ferrocene and corannulene templates

Abstract:
The smallest and most strained member of a family of π-conjugated cyclic porphyrin oligomers was synthesized by using pentapyridyl templates based on ferrocene and corannulene. Both templates are effective for directing the synthesis of the butadiyne-linked cyclic pentamer, despite the fact that the radii of their N5 donor sets are too small by 0.5 Å and 0.9 Å, respectively (from DFT calculations). The five-porphyrin nanoring exhibits a structured absorption spectrum and its fluorescence extends to 1200 nm, reflecting strong π conjugation and Herzberg-Teller vibronic coupling.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1002/anie.201602909

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author


Publisher:
Wiley
Journal:
Angewandte Chemie International Edition More from this journal
Volume:
55
Issue:
29
Pages:
8358-8362
Publication date:
2016-05-23
Acceptance date:
2016-04-14
DOI:
EISSN:
1521-3773
ISSN:
1433-7851


Language:
English
Keywords:
Pubs id:
pubs:625194
UUID:
uuid:c151ba7c-a44a-4271-b831-fc1cd95f6d70
Local pid:
pubs:625194
Source identifiers:
625194
Deposit date:
2016-06-10

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