Journal article icon

Journal article

Ni(2,2′:6′,2′′-terpyridine) 2: a high-spin octahedral formal Ni(0) complex †

Abstract:
We have synthesised and characterised the complex Ni(tpy)2 (tpy = 2,2′:6′,2′′-terpyridine). This formally Ni(0) complex is paramagnetic both in the solid state and in solution (S = 2). The crystal structure shows an octahedral geometry, with molecules arranged in independent dimers involving π-stacking between pairs of complexes. Magnetic measurementes and DFT calculations suggest the existence of temperature-dependent intermolecular antiferromagnetic coupling in the solid state.
Publication status:
Published
Peer review status:
Peer reviewed

Actions


Access Document


Publisher copy:
10.1039/d3dt04247b

Authors


More by this author
Role:
Author
ORCID:
0000-0002-1552-0901
More by this author
Institution:
University of Oxford
Role:
Author


More from this funder
Funder identifier:
https://ror.org/01cwqze88
More from this funder
Funder identifier:
https://ror.org/05r0vyz12


Publisher:
Royal Society of Chemistry
Journal:
Dalton Transactions More from this journal
Publication date:
2024-05-01
Acceptance date:
2024-04-16
DOI:
EISSN:
1477-9234
ISSN:
1477-9226


Language:
English
Source identifiers:
1950485
Deposit date:
2024-07-20

Terms of use



Views and Downloads






If you are the owner of this record, you can report an update to it here: Report update to this record

TO TOP