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Optimising adsorptive stripping voltammetry: strategies and limitations

Abstract:
The widely employed electroanalytical technique of adsorptive stripping voltammetry (AdsSV) is critically assessed and evaluated at a wide and diverse range of unmodified and nano-particle modified carbon electrodes using the analyte fipronil as a paradigmatic case. The generic electroanalytical performances of the nano-particle modified electrodes are investigated and compared with the unmodified electrodes revealing similar LOD values and pointing to intrinsic limitations of AdsSV arising from the non-independence of the Faradaic and capacitive signals during the stripping step. Methods for facilitating the adsorption or using different waveforms that may offer a more favourable limit of detection (LOD) at the nano-particle modified electrodes are suggested and assessed, specifically the use of adsorption onto particles prior to their use for modifying electrodes and also the recently introduced method of semi-circular voltammetry.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1002/celc.202100679

Authors

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Oxford college:
Wadham College
Role:
Author


Publisher:
Wiley
Journal:
ChemElectroChem More from this journal
Volume:
8
Issue:
12
Pages:
2343-2352
Publication date:
2021-06-09
Acceptance date:
2021-06-09
DOI:
EISSN:
2196-0216


Language:
English
Keywords:
Pubs id:
1182220
Local pid:
pubs:1182220
Deposit date:
2021-06-16
ARK identifier:

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