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Crystal structure and magnetic modulation in beta-Ce2O2FeSe2

Abstract:
We report a combination of X-ray and neutron diffraction studies, Mössbauer spectroscopy and muon spin relaxation (μ+SR) measurements to probe the structure and magnetic properties of the semiconducting β-Ce2O2FeSe2 oxychalcogenide. We report a new structural description in space group Pna21 which is consistent with diffraction data and second harmonic generation measurements and reveal an order-disorder transition on one Fe site at TOD ≈ 330 K. Susceptibility measurements, Mössbauer and μ+SR reveal antiferromagnetic ordering below TN = 86 K and more complex short range order above this temperature. 12 K neutron diffraction data reveal a modulated magnetic structure with q = 0.444 bN*
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/PhysRevMaterials.1.034403

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Funder identifier:
https://ror.org/0439y7842
Grant:
EP/N024028/1


Publisher:
American Physical Society
Journal:
Physical Review Materials More from this journal
Volume:
1
Issue:
3
Article number:
034403
Publication date:
2017-08-11
Acceptance date:
2017-06-30
DOI:
EISSN:
2475-9953


Language:
English
Pubs id:
pubs:812123
UUID:
uuid:bd41ea6c-6bbb-4599-9790-1bd3e928a2ac
Local pid:
pubs:812123
Source identifiers:
812123
Deposit date:
2018-04-09

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