- Abstract:
-
We report the one-pot, solvent free synthesis of a stimuli-responsive polyurethane (PU) adhesive. The hard domains within the supramolecular PU network contain a silyl protected phenol ‘degradable unit’ (DU). The DU undergoes rapid decomposition (<30 minutes) upon treatment with fluoride ions which causes depolymerisation of the linear PU adhesive. The mechanism of depolymerisation was investigated in solution using 1H NMR spectroscopy by following the degradation of the polymer in the pre...
Expand abstract - Publication status:
- Published
- Peer review status:
- Peer reviewed
- Version:
- Accepted Manuscript
- Files:
-
-
(pdf, 1.2MB)
-
(pdf, 1.8MB)
-
- Publisher copy:
- 10.1039/C7PY01653K
-
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- Funding agency for:
- Babra, TS
- Funding agency for:
- Trivedi, A
- Publisher:
- Royal Society of Chemistry Publisher's website
- Journal:
- Polymer Chemistry Journal website
- Volume:
- 46
- Issue:
- 8
- Pages:
- 7207-7216
- Publication date:
- 2017-11-14
- Acceptance date:
- 2017-11-05
- DOI:
- EISSN:
-
1759-9962
- ISSN:
-
1759-9954
- Pubs id:
-
pubs:745710
- URN:
-
uri:b98d2509-e3ec-4563-8ded-2853c156a55d
- UUID:
-
uuid:b98d2509-e3ec-4563-8ded-2853c156a55d
- Local pid:
- pubs:745710
- Copyright holder:
- Babra, et al
- Copyright date:
- 2017
- Notes:
- © Babra, et al 2017. This is the author accepted manuscript following peer review version of the article. The final version is available online from Royal Society of Chemistry at: 10.1039/C7PY01653K
Journal article
Fluoride degradable and thermally debondable polyurethane based adhesive
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+ Engineering and Physical Sciences Research Council
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+ Air Force Office of Scientific Research, Air Force Material Command, USAF
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