Journal article icon

Journal article

Catalysis and tunnelling in the unimolecular decay of Criegee intermediates

Abstract:
The unimolecular decay of Criegee intermediates is the major producer of OH radicals in the atmosphere. Here, Semi-Classical Transition State Theory (SCTST) in full and reduced dimensions is used to determine thermal rate constants for their unimolecular decay, as well as their decay catalysed by a single water molecule. These reactions shed light on the applicability of SCTST for catalysed hydrogen transfer reactions.
Publication status:
Published
Peer review status:
Peer reviewed

Actions


Access Document


Files:
Publisher copy:
10.1039/c8cp05021j

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Oxford college:
Brasenose College
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Oxford college:
Magdalen College
Role:
Author
ORCID:
0000-0003-4439-741X


More from this funder
Funding agency for:
Shan, X
Clary, D
Grant:
RPG-2013-321
RPG-2013-321


Publisher:
Royal Society of Chemistry
Journal:
Physical Chemistry Chemical Physics More from this journal
Volume:
20
Pages:
25224-25234
Publication date:
2018-09-25
Acceptance date:
2018-09-24
DOI:
EISSN:
1463-9084
ISSN:
1463-9076
Pmid:
30264080


Language:
English
Pubs id:
pubs:923794
UUID:
uuid:b7d2d2ba-65f4-48a4-a66a-c6d801e895e1
Local pid:
pubs:923794
Source identifiers:
923794
Deposit date:
2018-10-22

Terms of use



Views and Downloads






If you are the owner of this record, you can report an update to it here: Report update to this record

TO TOP