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Synthesis of metallophosphaalkenes by reaction of organometallic nucleophiles with a phosphaethynolato-borane

Abstract:
We describe the reaction of a phosphaethynolato-borane [B]OCP ([B] = N,N′-bis(2,6-diisopropylphenyl)-2,3-dihydro-1H-1,3,2-diazaboryl) with the organometallic nucleophile Na[Cp*Fe(CO)2] (Cp* = pentamethylcyclopentadienyl). The electrophilic character of [B]OCP allows for a new route towards the formation metal–phosphorus bonds affording a metallophosphaalkene that can be functionalised at both the oxygen and phosphorus atoms depending on the reagents employed.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1039/c9cc03040a

Authors

More by this author
Institution:
University of Oxford
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
ORCID:
0000-0002-4532-0329
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Oxford college:
Lady Margaret Hall
Role:
Author
ORCID:
0000-0002-7311-1663


Publisher:
Royal Society of Chemistry
Journal:
Chemical Communications More from this journal
Volume:
55
Issue:
48
Pages:
6842-6845
Publication date:
2019-05-14
Acceptance date:
2019-05-14
DOI:
EISSN:
1364-548X
ISSN:
1359-7345
Pmid:
31120468


Language:
English
Keywords:
Pubs id:
pubs:1003293
UUID:
uuid:b41e2a5a-7208-421b-b7da-67b333dd2fcb
Local pid:
pubs:1003293
Source identifiers:
1003293
Deposit date:
2019-05-31
ARK identifier:

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