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Dynamics of individual Brownian rods in a microchannel flow

Abstract:
We study the orientational dynamics of heavy silica microrods flowing through a microfluidic channel. Comparing experiments and Brownian dynamics simulations we identify different particle orbits, in particular in-plane tumbling behavior, which cannot be explained by classical Jeffery theory, and we relate this behavior to the rotational diffusion of the rods. By constructing the full, three-dimensional, orientation distribution, we describe the rod trajectories and quantify the persistence of Jeffery orbits using temporal correlation functions of the Jeffery constant. We find that our colloidal rods lose memory of their initial configuration in about a second, corresponding to half a Jeffery period.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1039/c9sm00903e

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Physics
Sub department:
Theoretical Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Physics
Sub department:
Theoretical Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Physics
Sub department:
Theoretical Physics
Role:
Author


Publisher:
Royal Society of Chemistry
Journal:
Soft Matter More from this journal
Volume:
15
Pages:
5810-5814
Publication date:
2019-07-09
Acceptance date:
2019-07-09
DOI:
EISSN:
1744-6848
ISSN:
1744-683X


Pubs id:
pubs:1032349
UUID:
uuid:ae2a6e64-fff0-4657-9e07-a8ff9e332adc
Local pid:
pubs:1032349
Source identifiers:
1032349
Deposit date:
2019-07-16

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