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Femtosecond broadband stimulated Raman spectroscopy: Apparatus and methods.

Abstract:

The laser, detection system, and methods that enable femtosecond broadband stimulated Raman spectroscopy (FSRS) are presented in detail. FSRS is a unique tool for obtaining high time resolution (<100 fs) vibrational spectra with an instrument response limited frequency resolution of <10 cm(-1). A titanium:Sapphire-based laser system produces the three different pulses needed for FSRS: (1) A femtosecond visible actinic pump that initiates the photochemistry, (2) a narrow bandwidth picose...

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Publication status:
Published

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Publisher copy:
10.1063/1.1807566

Authors


McCamant, DW More by this author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Mathies, RA More by this author
Journal:
The Review of scientific instruments
Volume:
75
Issue:
11
Pages:
4971-4980
Publication date:
2004-11-05
DOI:
EISSN:
1089-7623
ISSN:
0034-6748
URN:
uuid:a9ab5dc9-2b01-4f1a-a9c5-3d956632c805
Source identifiers:
118468
Local pid:
pubs:118468
Language:
English

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