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High irradiance performance of metal halide perovskites for concentrator photovoltaics

Abstract:
Traditionally, III–V multi-junction cells have been used in concentrator photovoltaic (CPV) applications, which deliver extremely high efficiencies but have failed to compete with ‘flat-plate’ silicon technologies owing to cost. Here, we assess the feasibility of using metal halide perovskites for CPVs, and we evaluate their device performance and stability under concentrated light. Under simulated sunlight, we achieve a peak efficiency of 23.6% under 14 Suns (that is, 14 times the standard solar irradiance), as compared to 21.1% under 1 Sun, and measure 1.26 V open-circuit voltage under 53 Suns, for a material with a bandgap of 1.63 eV. Importantly, our encapsulated devices maintain over 90% of their original efficiency after 150 h aging under 10 Suns at maximum power point. Our work reveals the potential of perovskite CPVs, and may lead to new PV deployment strategies combining perovskites with low-concentration factor and lower-accuracy solar tracking systems.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1038/s41560-018-0220-2

Authors


More by this author
Institution:
University of Oxford
Division:
Maths, Physical & Life Sciences
Department:
Condensed Matter Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
Maths, Physical & Life Sciences
Department:
Condensed Matter Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
Maths, Physical & Life Sciences
Department:
Condensed Matter Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
Maths, Physical & Life Sciences
Department:
Condensed Matter Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
Maths, Physical & Life Sciences
Department:
Condensed Matter Physics
Role:
Author


Publisher:
Nature Publishing Group
Journal:
Nature Energy More from this journal
Volume:
3
Pages:
855–861
Publication date:
2018-08-06
Acceptance date:
2018-07-05
DOI:
EISSN:
2058-7546


Keywords:
Pubs id:
pubs:897007
UUID:
uuid:a4bd4bf9-7759-44d0-a7ca-6127737eb12b
Local pid:
pubs:897007
Source identifiers:
897007
Deposit date:
2018-08-09

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