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Organocatalytic highly enantioselective conjugate addition of aldehydes to alkylidine malonates

Abstract:
The first highly enantioselective, direct organocatalytic conjugate addition of unmodified aldehydes to alkylidinemalonates is presented. The reaction gives access to β-formyl-substituted malonates and highly functionalized lactones with up to 14:1 dr and generally 94 to >99% ee. © 2008 Wiley-VCH Verlag GmbH and Co. KGaA.
Publication status:
Published

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Publisher copy:
10.1002/adse.200700570

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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Inorganic Chemistry
Role:
Author
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Journal:
ADVANCED SYNTHESIS and CATALYSIS
Volume:
350
Issue:
5
Pages:
657-661
Publication date:
2008-03-05
DOI:
EISSN:
1521-3897
ISSN:
1615-4150
URN:
uuid:a2af7585-ba59-4658-a09e-cf810475d9fe
Source identifiers:
321986
Local pid:
pubs:321986

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