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PdIn intermetallic nanoparticles for the hydrogenation of CO2 to methanol

Abstract:

Direct hydrogenation of CO2 to methanol could offer significant environmental benefits, if efficient catalysts can be developed. Here, bimetallic Pd-In nanoparticles show good performance as catalysts for this reaction. Unsupported nanoparticles are synthesised by the thermal decomposition of Pd(acetate)2 and In(acetate)3 precursors in a high boiling point solvent (squalane), followed by reduction using dilute H2 gas (210 °C). Adjusting the ratio of the two metallic precursors allow access to...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Publisher's version

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Publisher copy:
10.1016/j.apcatb.2017.07.069

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Department:
Oxford, MPLS, Chemistry
Regoutz, A More by this author
Shaffer, M More by this author
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Grant:
EP/H046380, EP/K035274/1, EP/M013839/1, EP/M028291/1
Publisher:
Elsevier Publisher's website
Journal:
Applied Catalysis B: Environmental Journal website
Volume:
220
Pages:
9-18
Publication date:
2017-07-25
Acceptance date:
2017-07-24
DOI:
ISSN:
0926-3373
Pubs id:
pubs:710885
URN:
uri:9f74005e-fda0-4445-a4cd-753a3c103554
UUID:
uuid:9f74005e-fda0-4445-a4cd-753a3c103554
Local pid:
pubs:710885

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