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Template-directed synthesis of a conjugated zinc porphyrin nanoball

Abstract:
We report the template-directed synthesis of a π-conjugated 14-porphyrin nanoball. This structure consists of two intersecting nanorings containing six and 10 porphyrin units. Fluorescence upconversion spectroscopy experiments demonstrate that electronic excitation delocalizes over the whole three-dimensional π system in less than 0.3 ps if the nanoball is bound to its templates or over 2 ps if the nanoball is empty.
Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted Manuscript

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Publisher copy:
10.1021/jacs.8b02552

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Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Role:
Author
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Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Role:
Author
ORCID:
0000-0002-6107-2310
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Institution:
University of Oxford
Division:
MPLS Division
Department:
Physics
Role:
Author
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Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Role:
Author
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Engineering and Physical Sciences Research Council More from this funder
Publisher:
American Chemical Society Publisher's website
Journal:
Journal of the American Chemical Society Journal website
Volume:
140
Issue:
16
Pages:
5352-5355
Publication date:
2018-04-11
Acceptance date:
2018-04-11
DOI:
EISSN:
1520-5126
ISSN:
0002-7863
Pubs id:
pubs:843486
URN:
uri:9b9f4aca-c8e2-4f3f-99be-c4332413930e
UUID:
uuid:9b9f4aca-c8e2-4f3f-99be-c4332413930e
Local pid:
pubs:843486
Language:
English

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