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Dynamical screening in SrVO3: Inelastic x-ray scattering experiments and ab initio calculations

Abstract:
We characterize experimentally and theoretically the high-energy dielectric screening properties of the prototypical correlated metal SrVO3. The dynamical structure factor measured by inelastic x-ray scattering spectroscopy as a function of momentum transfer is in very good agreement with first-principles calculations in the adiabatic local-density approximation to time-dependent density-functional theory. Our results reveal the crucial importance of crystal local fields in the charge response function of correlated materials: They lead to depolarization effects for localized excitations and couple spectra from different Brillouin zones.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/PhysRevB.103.235136

Authors



Publisher:
American Physical Society
Journal:
Physical Review B More from this journal
Volume:
103
Issue:
23
Article number:
235136
Publication date:
2021-06-16
Acceptance date:
2021-05-25
DOI:
EISSN:
2469-9969
ISSN:
2469-9950


Language:
English
Keywords:
Pubs id:
1185754
Local pid:
pubs:1185754
Deposit date:
2021-08-04

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