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Vapor pressure and heat of vaporization of molecules that associate in the gas phase

Abstract:
A model of the temperature dependence of the vapor pressure and the heat of vaporization of liquids whose vapors contain associates is presented for two cases: dimers and linear associates in the gas phase. The results are analytic generalizations of the Clausius–Clapeyron equation, valid with accuracy of 0.1%–1%, as demonstrated with 11 liquids: formic and acetic acids, methanol, ethanol, n-propanol, n-butanol, water, benzene, toluene, heptane, and isooctane. The model involves only readily available handbook parameters: the room-temperature heat of vaporization, vapor pressure, heat capacities, second virial coefficient, and heat of dissociation of the dimers in the gas phase.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/acs.iecr.7b04241

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author


Publisher:
American Chemical Society
Journal:
Industrial and Engineering Chemistry Research More from this journal
Volume:
57
Issue:
16
Pages:
5722–5731
Publication date:
2018-03-27
Acceptance date:
2018-03-27
DOI:
ISSN:
0888-5885


Keywords:
Pubs id:
pubs:843978
UUID:
uuid:969b22d4-d910-4981-8c0f-379e53ff9f02
Local pid:
pubs:843978
Source identifiers:
843978
Deposit date:
2018-04-24

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