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Evidence for a Jeff=0 ground state and defect-induced spin glass behavior in the pyrochlore osmate Y2Os2O7

Abstract:

We present AC and DC magnetometry, heat capacity, muon spin relaxation (μSR), and resonant inelastic x-ray scattering (RIXS) studies of the pyrochlore osmate Y2Os2O7. Consistent with previous results, we observe a small Curie-Weiss effective moment of approximately 0.4 μB and spin freezing at a temperature Tf≃5K. On the other hand, our analysis of the RIXS spectra with single-ion energy-level calculations implies a nonmagnetic Jeff=0 ground state on the Os4+ sites, with the spin-orbit interac...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/physrevb.99.174442

Authors


Publisher:
American Physical Society
Journal:
Physical Review B More from this journal
Volume:
99
Issue:
17
Article number:
174442
Publication date:
2019-05-31
Acceptance date:
2019-05-01
DOI:
EISSN:
2469-9969
ISSN:
2469-9950
Language:
English
Keywords:
Pubs id:
pubs:1020160
UUID:
uuid:966f16cf-18e0-4b82-adb1-f07ad58462d0
Local pid:
pubs:1020160
Source identifiers:
1020160
Deposit date:
2019-11-24

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