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Trifluoromethylation of allylsilanes under copper catalysis.

Abstract:
Branched allylic CF 3 products are accessible by copper-catalyzed trifluoromethylation of allylsilanes with the Togni reagent I. The silyl group is critical to control the outcome of this reaction because in its absence, a product of addition between the alkene and the Togni reagent is formed preferentially. The reaction is inhibited with 2,2,6,6-tetramethyl-1- piperidinyloxy (TEMPO) and is likely to operate via multiple reaction pathways. Copyright © 2012 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim.
Publication status:
Published

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Publisher copy:
10.1002/chem.201201707

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Journal:
Chemistry (Weinheim an der Bergstrasse, Germany) More from this journal
Volume:
18
Issue:
28
Pages:
8583-8587
Publication date:
2012-07-01
DOI:
EISSN:
1521-3765
ISSN:
0947-6539


Language:
English
Keywords:
Pubs id:
pubs:339836
UUID:
uuid:95ae5d32-5e01-44ec-acd8-eba2a844e0da
Local pid:
pubs:339836
Source identifiers:
339836
Deposit date:
2012-12-19
ARK identifier:

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