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Fine-tuning the local symmetry to attain record blocking temperature and magnetic remanence in a single-ion magnet

Abstract:

Remanence and coercivity are the basic characteristics of permanent magnets. They are also tightly correlated with the existence of long relaxation times of magnetization in a number of molecular complexes, called accordingly single-molecule magnets (SMMs). Up to now, hysteresis loops with large coercive fields have only been observed in polynuclear metal complexes and metal-radical SMMs. On the contrary, mononuclear complexes, called single-ion magnets (SIM), have shown hysteresis loops of b...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1002/anie.201310451

Authors


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Department:
Oxford, MPLS, Materials
Korobkov, I More by this author
Murugesu, M More by this author
Chibotaru, LF More by this author
Publisher:
Wiley Online Library Publisher's website
Journal:
Angewandte Chemie International Edition Journal website
Volume:
53
Issue:
17
Pages:
4413–4417
Publication date:
2014-03-20
DOI:
ISSN:
1433-7851
Pubs id:
pubs:652758
URN:
uri:8f34bc5a-a4e5-466e-bb11-1f20f1b1ad32
UUID:
uuid:8f34bc5a-a4e5-466e-bb11-1f20f1b1ad32
Local pid:
pubs:652758
Keywords:

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