Journal article

Charge-carrier dynamics in vapour-deposited films of the organolead halide perovskite CH3NH3PbI3-xClx

Abstract:: We determine high charge-carrier mobilities ≥ 33 cm2 V−1 s−1 and bi-molecular recombination rates about five orders of magnitude below the prediction of Langevin's model for vapour-deposited CH3NH3PbI3−xClx using ultrafast THz spectroscopy. At charge-carrier densities below ∼1017 cm−3 intrinsic diffusion lengths are shown to approach 3 microns, limited by slow mono-molecular decay processes.

Publication status:: Published

Peer review status:: Peer reviewed

Actions

Email

Email this record

Send the bibliographic details of this record to your email address.

Your Email
Please enter the email address that the record information will be sent to.

-
Your message (optional)
Please add any additional information to be included within the email.
Cite

Cite this record

APA Style

Wehrenfennig, C., Liu, M., Snaith, H., Johnston, M., & Herz, L. (2014). Charge-carrier dynamics in vapour-deposited films of the organolead halide perovskite CH3NH3PbI3-xClx. Energy and Environmental Science, 7(7), 2269–2275.

MLA Style

Wehrenfennig, C., et al. “Charge-Carrier Dynamics in Vapour-Deposited Films of the Organolead Halide Perovskite CH3NH3PbI3-XClx.” Energy and Environmental Science, vol. 7, no. 7, Royal Society of Chemistry, 2014, pp. 2269–75.

Chicago Style

Wehrenfennig, C, M Liu, H Snaith, M Johnston, and L Herz. 2014. “Charge-Carrier Dynamics in Vapour-Deposited Films of the Organolead Halide Perovskite CH3NH3PbI3-XClx.” Energy and Environmental Science 7 (7): 2269–75.
Share
Print

Access Document

Files:: Wehrenfennig et al, Charge-carrier dynamics in vapour-deposite...

(Preview, Accepted manuscript, pdf, 3.7MB, Terms of use)

Publisher copy:: 10.1039/c4ee01358a

Authors

+ Wehrenfennig, C More by this author

Role:: Author

+ Liu, M More by this author

Role:: Author

+ Snaith, H More by this author

Institution:: University of Oxford
Division:: MPLS
Department:: Physics
Sub department:: Condensed Matter Physics
Role:: Author

+ Johnston, M More by this author

Institution:: University of Oxford
Division:: MPLS
Department:: Physics
Sub department:: Condensed Matter Physics
Role:: Author

+ Herz, L More by this author

Institution:: University of Oxford
Division:: MPLS
Department:: Physics
Sub department:: Condensed Matter Physics
Role:: Author

+ Engineering and Physical Sciences Research Council More from this funder

Publisher:: Royal Society of Chemistry
Journal:: Energy and Environmental Science More from this journal
Volume:: 7
Issue:: 7
Pages:: 2269-2275
Publication date:: 2014-07-01
DOI:: 10.1039/c4ee01358a
EISSN:: 1754-5706
ISSN:: 1754-5692

Pubs id:: pubs:474087
UUID:: uuid:8ee16765-d52d-4a72-949b-f34e14f03b99
Local pid:: pubs:474087
Source identifiers:: 474087
Deposit date:: 2014-07-11

Terms of use

Copyright holder:: Royal Society of Chemistry
Copyright date:: 2014
Notes:: © The Royal Society of Chemistry 2014

Licence:: Terms and Conditions of Use for Oxford University Research Archive

Views and Downloads

About views and downloads

If you are the owner of this record, you can report an update to it here: Report update to this record

TO TOP