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Charge transport through extended molecular wires with strongly correlated electrons

Abstract:

Electron–electron interactions are at the heart of chemistry and understanding how to control them is crucial for the development of molecular-scale electronic devices. Here, we investigate single-electron tunneling through a redox-active edge-fused porphyrin trimer and demonstrate that its transport behavior is well described by the Hubbard dimer model, providing insights into the role of electron–electron interactions in charge transport. In particular, we empirically determine the molecule...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1039/D1SC03050G

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Institution:
University of Oxford
Role:
Author
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Name:
Engineering & Physical Sciences Research Council
Grant:
EP/N017188/1
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Name:
Engineering and Physical Sciences Research Council
Grant:
EP/R029229/1
Publisher:
Royal Society of Chemistry
Journal:
Chemical Science More from this journal
Volume:
12
Issue:
33
Pages:
11121-11129
Publication date:
2021-07-26
Acceptance date:
2021-07-19
DOI:
ISSN:
2041-6520
Language:
English
Keywords:
Pubs id:
1187218
Local pid:
pubs:1187218
Deposit date:
2021-07-21

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