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Thesis

Long-term degradation of lithium-ion batteries

Abstract:
In this thesis, we develop efficient mathematical models of lithium-ion batteries and the key degradation mechanism, solid–electrolyte interphase (SEI) growth. By doing this, we provide a modular mathematical framework for lithium-ion battery modelling from which an appropriate fidelity model can be selected and extended. Our approach is to develop detailed physics-based models motivated by standard electrochemical modelling approaches and then employ asymptotic methods to systematically simplify these models. An important output of this work is an open-source battery modelling software called PyBaMM (Python Battery Mathematical Modelling) that allows other researchers to easily use and interact with the models we develop.

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Division:
MPLS
Department:
Mathematical Institute
Role:
Author

Contributors

Role:
Supervisor
ORCID:
0000-0001-8917-8574
Role:
Supervisor
Role:
Examiner
ORCID:
0000-0001-6882-7977


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Funder identifier:
http://dx.doi.org/10.13039/501100000266
Grant:
EP/L015803/1)
Programme:
Engineering and Physical Sciences Research Council Centre For Doctoral Training in Industrially Focused Mathematical Modelling


Type of award:
DPhil
Level of award:
Doctoral
Awarding institution:
University of Oxford


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