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Low-temperature magnetism of KAgF3

Abstract:

KAgF3 is a quasi-one-dimensional quantum antiferromagnet hosting a series of intriguing structural and magnetic transitions. Here we use powder neutron diffraction, μSR spectroscopy, and density functional theory calculations to elucidate the low-temperature magnetic phases. Below TN1 = 29 K we find that the material orders as an A-type antiferromagnet with an ordered moment of 0.52 μ B . Both neutrons and muons provide evidence for an intermediate phase at temperatures TN1 < T < TN2 with TN2 ≈ 66 K from a previous magnetometry study. However, the evidence is at the limit of detection and its nature remains an open problem.

Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/PhysRevB.107.144422

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Role:
Author
ORCID:
0000-0001-6879-7181
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Oxford college:
Mansfield College
Role:
Author
ORCID:
0000-0002-3426-0834
More by this author
Role:
Author
ORCID:
0000-0001-7915-3453
More by this author
Role:
Author
ORCID:
0000-0002-9284-6585
More by this author
Role:
Author
ORCID:
0000-0003-4611-2393


Publisher:
American Physical Society
Journal:
Physical Review B More from this journal
Volume:
107
Issue:
14
Article number:
144422
Publication date:
2023-04-20
Acceptance date:
2023-03-30
DOI:
EISSN:
2469-9969
ISSN:
2469-9950


Language:
English
Keywords:
Pubs id:
1345044
Local pid:
pubs:1345044
Deposit date:
2023-06-09

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