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Formation of an artificial Mg2+-permeable interphase on Mg anodes compatible with ether and carbonate electrolytes

Abstract:

Rechargeable Mg-ion batteries typically suffer from either rapid passivation of the Mg anode or severe corrosion of the current collectors by halogens within the electrolyte, limiting their practical implementation. Here, we demonstrate the broadly applicable strategy of forming an artificial solid electrolyte interphase (a-SEI) layer on Mg to address these challenges. The a-SEI layer is formed by simply soaking Mg foil in a tetraethylene glycol dimethyl ether solution containing LiTFSI and A...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/acsami.0c22520

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Publisher:
American Chemical Society Publisher's website
Journal:
ACS Applied Materials and Interfaces Journal website
Volume:
13
Issue:
21
Pages:
24565–24574
Publication date:
2021-05-19
Acceptance date:
2021-04-21
DOI:
EISSN:
1944-8244
ISSN:
1944-8252
Pubs id:
1174496
Local pid:
pubs:1174496

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