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Formation mechanism for a hybrid supramolecular network involving cooperative interactions.

Abstract:

A novel mechanism of hybrid assembly of molecules on surfaces is proposed stemming from interactions between molecules and on-surface metal atoms which eventually got trapped inside the network pores. Based on state-of-the-art theoretical calculations, we find that the new mechanism relies on formation of molecule-metal atom pairs which, together with molecules themselves, participate in the assembly growth. Most remarkably, the dissociation of pairs is facilitated by a cooperative interactio...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted manuscript

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Institution:
University of Oxford
Department:
Oxford, MPLS, Materials
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Materials
Role:
Author
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Materials
Role:
Author
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Publisher:
American Physical Society Publisher's website
Journal:
Physical Review Letters Journal website
Volume:
108
Issue:
17
Pages:
176103
Chapter number:
ARTN 176103
Publication date:
2012-04-27
DOI:
EISSN:
1079-7114
ISSN:
0031-9007
URN:
uuid:785a3a3c-fa2e-4d46-a23a-02ac17f0be10
Source identifiers:
333646
Local pid:
pubs:333646
Language:
English

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