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Journal article

Weak liquid water path response in ship tracks

Abstract:

The assessment of aerosol–cloud interactions remains a major source of uncertainty in understanding climate change, partly due to the difficulty in making accurate observations of aerosol impacts on clouds. Ships can release large numbers of aerosols that serve as cloud condensation nuclei, which can create artificially brightened clouds known as ship tracks. These aerosol emissions offer a “natural”, or “opportunistic”, experiment to explore aerosol effects on clouds, while also disentangling meteorological influences. Utilizing ship positions and reanalysis wind fields, we predict ship track locations, colocating them with satellite data to depict the temporal evolution of cloud properties after an aerosol perturbation. Repeating our analysis for a null experiment does not necessarily recover zero signal as expected; instead, it reveals subtleties between different null-experiment methodologies. This study uncovers a systematic bias in prior ship track research, due to the assumption that background gradients will, on average, be linear. We correct for this bias, which is linked to the correlation between wind fields and cloud properties, to reveal the true ship track response.

We find that, once this bias is corrected for, the liquid water path (LWP) response after an aerosol perturbation is weak on average. This has important implications for estimates of radiative forcings due to LWP adjustments, as previous responses in unstable cases were overestimated. A noticeable LWP response is only recovered in specific cases, such as marine stratocumulus clouds, where a positive LWP response is found in precipitating or clean clouds. This work highlights subtleties in the analysis of isolated opportunistic experiments, reconciling differences in the LWP response to aerosols reported in previous studies.

Publication status:
Published
Peer review status:
Peer reviewed

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Files:
Publisher copy:
10.5194/acp-24-13269-2024

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Role:
Author


More from this funder
Funder identifier:
https://ror.org/00k4n6c32
Grant:
860100
821205
More from this funder
Funder identifier:
https://ror.org/02b5d8509
Grant:
NE/S005099/1


Publisher:
European Geosciences Union
Journal:
Atmospheric Chemistry and Physics More from this journal
Volume:
24
Issue:
23
Pages:
13269-13283
Publication date:
2024-12-02
Acceptance date:
2024-10-01
DOI:
EISSN:
1680-7324
ISSN:
1680-7316


Language:
English
Pubs id:
2068110
Local pid:
pubs:2068110
Deposit date:
2024-12-02

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