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Journal article

A fast microchannel plate-scintillator detector for velocity map imaging and imaging mass spectrometry.

Abstract:
The time resolution achievable using standard position-sensitive ion detectors, consisting of a chevron pair of microchannel plates coupled to a phosphor screen, is primarily limited by the emission lifetime of the phosphor, around 70 ns for the most commonly used P47 phosphor. We demonstrate that poly-para-phenylene laser dyes may be employed extremely effectively as scintillators, exhibiting higher brightness and much shorter decay lifetimes than P47. We provide an extensive characterisation of the properties of such scintillators, with a particular emphasis on applications in velocity-map imaging and microscope-mode imaging mass spectrometry. The most promising of the new scintillators exhibits an electron-to-photon conversion efficiency double that of P47, with an emission lifetime an order of magnitude shorter. The new scintillator screens are vacuum stable and show no signs of signal degradation even over longer periods of operation.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1063/1.4866647

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Chemistry Research Laboratory
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Chemistry Research Laboratory
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author


More from this funder
Funding agency for:
Vallance, C
Grant:
238671
More from this funder
Funding agency for:
Brouard, M
Vallance, C
Grant:
238671
238671
More from this funder
Funding agency for:
Brouard, M
Vallance, C
Grant:
238671
238671
More from this funder
Funding agency for:
Brouard, M
Vallance, C
Grant:
238671
238671
More from this funder
Funding agency for:
Brouard, M
Vallance, C
Grant:
238671
238671


Publisher:
AIP Publishing LLC
Journal:
Review of scientific instruments More from this journal
Volume:
85
Issue:
2
Pages:
023306
Publication date:
2014-02-28
DOI:
EISSN:
1089-7623
ISSN:
0034-6748


Language:
English
Pubs id:
pubs:451121
UUID:
uuid:71a382be-9625-49f2-b5bb-b20c8948ae78
Local pid:
pubs:451121
Source identifiers:
451121
Deposit date:
2014-05-13

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