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The reductive C3-functionalisation of pyridinium and quinolinium salts through iridium-catalysed interrupted transfer hydrogenation

Abstract:

This paper describes the transformation of flat N-containing aromatic compounds (pyridines and quinolines) into complex 3-dimensional heterocycles bearing new functionality which are ideal for further manipulation. In this reaction methanol and formaldehyde are used as starting materials for the reduction and functionalisation of arenes using an iridium catalyst; thus, inexpensive and renewable feedstocks are utilised in the rapid formation of complex and high value N-heterocycles. By harness...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted Manuscript

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Publisher copy:
10.1038/s41557-018-0178-5

Authors


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Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Subgroup:
Organic Chemistry
Oxford college:
Linacre College
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Subgroup:
Organic Chemistry
Oxford college:
Wolfson College
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Subgroup:
Organic Chemistry
Oxford college:
Keble College
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Lindsay-Scott, P More by this author
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Publisher:
Springer Nature Publisher's website
Journal:
Nature Chemistry Journal website
Volume:
11
Pages:
242–247
Publication date:
2018-12-17
Acceptance date:
2018-10-24
DOI:
EISSN:
1755-4349
ISSN:
1755-4330
Pubs id:
pubs:941336
URN:
uri:7143aeb5-2e3b-4a08-8813-d95ec205de3b
UUID:
uuid:7143aeb5-2e3b-4a08-8813-d95ec205de3b
Local pid:
pubs:941336

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