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Improved direct detection of low-energy ions using a multipixel photon counter coupled with a novel scintillator

Abstract:
All rights reserved.Recently, we described a direct low-energy ion detector for time-of-flight applications based on a single-photon avalanche diode (SPAD) array optically coupled to an LYSO (cerium-doped lutetium yttrium orthosilicate) scintillator. Here, we present a greatly improved version of the detector, developed through testing of a number of different scintillator and phosphor materials in combination with a commercially available SPAD array. The various scintillator materials have been characterized in terms of the achievable detection sensitivity and time response when used in conjunction with the SPAD array. Organic para-polyphenylene dyes, a relatively new class of scintillator for particle detection, were found to exhibit markedly improved performance relative to well-established scintillators such as LYSO crystal scintillators and P47 phosphors, both in terms of brightness and time response. The optimized detector has a time resolution of ∼2 ns, an improvement of more than an order of magnitude over the original version, at the same time as achieving a five- to ten-fold improvement in detection sensitivity. Our approach points the way towards the development of a generic silicon-based ion detector technology to complement or replace the microchannel-plate (MCP) ion detectors in widespread use at present. Such a detector would remove the need for high voltages and high vacuum, and at the same time greatly reduce detector cost relative to MCP-based detectors.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1016/j.ijms.2016.01.005

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author


Publisher:
Elsevier
Journal:
International Journal of Mass Spectrometry More from this journal
Volume:
397-398
Pages:
27-31
Publication date:
2016-02-01
Acceptance date:
2016-01-21
DOI:
ISSN:
1387-3806


Keywords:
Pubs id:
pubs:612057
UUID:
uuid:6cf78ace-ecce-43a9-9975-3b1330b9133c
Local pid:
pubs:612057
Source identifiers:
612057
Deposit date:
2016-11-01

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