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The influence of subwavelength geometry on extracting the electrical properties of semiconductors by terahertz spectroscopy

Abstract:
Terahertz (THz) spectroscopy is a non-contact technique well-suited for probing the ultrafast electrical conductivity of semiconductor nanostructures, where conventional methods are often impractical. However, geometric resonances in these nanostructures can distort the measured THz response, complicating the extraction of the intrinsic material properties. Here, we use THz spectroscopy to study GaAs nanowires of varying lengths and observe that the resonant frequency increases as the nanowire length decreases. Further measurements on a model system of well-defined GaAs microsquares (ranging in size from 500 × 500 to 7 × 7 μm2) confirmed the relationship between structure size and resonant frequency. We verify that a plasmon-based model successfully separates the geometric response from the intrinsic charge-carrier response. Thus, the model allows for the accurate evaluation of critical material properties in nanostructured semiconductors, such as electron mobility. Fluence-dependent measurements and finite-difference time-domain simulations confirm the plasmonic nature of the resonances.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1063/5.0273919

Authors

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Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
ORCID:
0009-0008-0136-6086
More by this author
Role:
Author
ORCID:
0000-0001-6033-7391
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
ORCID:
0000-0002-9201-9096
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
ORCID:
0000-0002-9933-8831
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
ORCID:
0000-0002-2111-3341


More from this funder
Funder identifier:
https://ror.org/05mmh0f86
Grant:
CE200100010
More from this funder
Funder identifier:
https://ror.org/0439y7842
Grant:
EP/T025077/1
EP/W018489/1


Publisher:
American Institute of Physics
Journal:
APL Photonics More from this journal
Volume:
10
Issue:
7
Article number:
076123
Publication date:
2025-07-28
Acceptance date:
2025-06-28
DOI:
EISSN:
2378-0967


Language:
English
Pubs id:
2133223
Local pid:
pubs:2133223
Deposit date:
2025-06-29
ARK identifier:

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