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The eutectic point in choline chloride and ethylene glycol mixtures

Abstract:
The choline chloride (ChCl) and ethylene glycol (EG) mixture has become established as a paradigmatic deep eutectic solvent (DES). Here, we present measurements of the phase behaviour of this mixture over a wide composition range, and provide an extended phase diagram. The eutectic point was found to lie at −28 ± 1 °C and 0.01 < xChCl < 0.02, sharply contrasting with the previously expected eutectic composition. Our observations confirm that the eutectic temperature is not ‘deep’ compared to the ideal solution theory prediction. We also observe a cold-crystallisation at T = −65 °C which may have been formerly misinterpreted as the eutectic point.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1039/d2cc04008e

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
ORCID:
0000-0002-0626-1522
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Oxford college:
Trinity College
Role:
Author
ORCID:
0000-0002-5875-5217


Publisher:
Royal Society of Chemistry
Journal:
Chemical Communications More from this journal
Volume:
58
Issue:
91
Pages:
12728-12731
Place of publication:
England
Publication date:
2022-10-26
Acceptance date:
2022-10-24
DOI:
EISSN:
1364-548X
ISSN:
1359-7345
Pmid:
36314432


Language:
English
Keywords:
Pubs id:
1300687
Local pid:
pubs:1300687
Deposit date:
2024-02-29

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