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Vibrational effects in charge transport through a molecular double quantum dot

Abstract:
Recent progress in the field of molecular electronics has revealed the fundamental importance of the coupling between the electronic degrees of freedom and specific vibrational modes. Considering the examples of a molecular dimer and a carbon nanotube double quantum dot, we here theoretically investigate transport through a two-site system that is strongly coupled to a single vibrational mode. Using a quantum master equation approach, we demonstrate that, depending on the relative positions of the two dots, electron-phonon interactions can lead to negative differential conductance and suppression of the current through the system. We also discuss the experimental relevance of the presented results and possible implementations of the studied system.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/PhysRevB.95.085423

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Materials
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Materials
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Materials
Role:
Author



Publisher:
American Physical Society
Journal:
Physical Review B More from this journal
Volume:
95
Issue:
085423
Pages:
1-11
Publication date:
2017-02-17
Acceptance date:
2017-01-26
DOI:
EISSN:
2469-9969
ISSN:
2469-9950


Keywords:
Pubs id:
pubs:673147
UUID:
uuid:65486074-8d88-46bf-8edd-f445daae19f5
Local pid:
pubs:673147
Source identifiers:
673147
Deposit date:
2017-02-06

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