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Journal article

Unveiling aerosol–cloud interactions – Part 1: Cloud contamination in satellite products enhances the aerosol indirect forcing estimate

Abstract:
Increased concentrations of aerosol can enhance the albedo of warm low-level cloud. Accurately quantifying this relationship from space is challenging due in part to contamination of aerosol statistics near clouds. Aerosol retrievals near clouds can be influenced by stray cloud particles in areas assumed to be cloud-free, particle swelling by humidification, shadows and enhanced scattering into the aerosol field from (3-D radiative transfer) clouds. To screen for this contamination we have developed a new cloud–aerosol pairing algorithm (CAPA) to link cloud observations to the nearest aerosol retrieval within the satellite image. The distance between each aerosol retrieval and nearest cloud is also computed in CAPA.

Results from two independent satellite imagers, the Advanced Along-Track Scanning Radiometer (AATSR) and Moderate Resolution Imaging Spectroradiometer (MODIS), show a marked reduction in the strength of the intrinsic aerosol indirect radiative forcing when selecting aerosol pairs that are located farther away from the clouds (−0.28±0.26 W m−2) compared to those including pairs that are within 15 km of the nearest cloud (−0.49±0.18 W m−2). The larger aerosol optical depths in closer proximity to cloud artificially enhance the relationship between aerosol-loading, cloud albedo, and cloud fraction. These results suggest that previous satellite-based radiative forcing estimates represented in key climate reports may be exaggerated due to the inclusion of retrieval artefacts in the aerosol located near clouds.

Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.5194/acp-17-13151-2017

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Atmos Ocean & Planet Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Physics; Atmos Ocean & Planet Physics
Role:
Author


More from this funder
Grant:
National Centre for Earth Observation
More from this funder
Grant:
theCloud_cci(contract:4000109870/13/I-NB)
LivingPlanetFellowship
theAerosol_cciprojects(ESAContractNo.4000109874/14/I-NB


Publisher:
European Geosciences Union
Journal:
Atmospheric Chemistry and Physics More from this journal
Volume:
17
Issue:
21
Pages:
13151-13164
Publication date:
2017-11-07
Acceptance date:
2017-09-12
DOI:
EISSN:
1680-7324
ISSN:
1680-7316


Pubs id:
pubs:746204
UUID:
uuid:64e7bbda-899f-4bd7-804e-a1f37fe3f130
Local pid:
pubs:746204
Source identifiers:
746204
Deposit date:
2017-11-17

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