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Uncovering Relationships between the Electronic Self-Energy and Coupled-Cluster Doubles Theory

Abstract:
We derive the coupled-cluster doubles (CCD) amplitude equations by introduction of the particle-hole-time decoupled electronic self-energy. The resulting analysis leads to an expression for the ground-state correlation energy that is exactly of the form obtained in coupled-cluster doubles theory. We demonstrate the relationship to the ionization potential/electron affinity equation-of-motion coupled-cluster doubles (IP/EA-EOM-CCD) eigenvalue problem by coupling the reverse-time self-energy contributions while maintaining particle-hole separability. The formal relationships established are demonstrated by exact solution of the Hubbard dimer.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/acs.jpca.5c03750

Authors

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Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Physics - Central
Role:
Author
ORCID:
0000-0003-3044-2224


Publisher:
American Chemical Society
Journal:
The Journal of Physical Chemistry A More from this journal
Volume:
129
Issue:
37
Pages:
8689-8698
Publication date:
2025-09-10
Acceptance date:
2025-08-25
DOI:
EISSN:
1520-5215
ISSN:
1089-5639


Language:
English
Pubs id:
2301254
Local pid:
pubs:2301254
Source identifiers:
3296872
Deposit date:
2025-09-19
ARK identifier:
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