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Magnetic excitations of the classical spin liquid MgCr2O4

Abstract:
We report a comprehensive inelastic neutron-scattering study of the frustrated pyrochlore antiferromagnet MgCr2O4 in its cooperative paramagnetic regime. Theoretical modeling yields a microscopic Heisenberg model with exchange interactions up to third-nearest neighbors, which quantitatively explains all the details of the dynamic magnetic response. Our work demonstrates that the magnetic excitations in paramagnetic MgCr2O4 are faithfully represented in the entire Brillouin zone by a theory of magnons propagating in a highly-correlated paramagnetic background. Our results also suggest that MgCr2O4 is proximate to a spiral spin-liquid phase distinct from the Coulomb phase, which has implications for the magneto-structural phase transition in MgCr2O4.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/PhysRevLett.122.097201

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Publisher:
American Physical Society
Journal:
Physical Review Letters More from this journal
Volume:
122
Issue:
9
Article number:
097201
Publication date:
2019-03-05
Acceptance date:
2019-02-12
DOI:
EISSN:
1079-7114
ISSN:
0031-9007


Pubs id:
pubs:976066
UUID:
uuid:5db3b1c2-4740-43e5-8a77-a0dc68b2a84f
Local pid:
pubs:976066
Source identifiers:
976066
Deposit date:
2019-02-27

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