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Underscreening in concentrated electrolyes

Abstract:

Screening of a surface charge by electrolyte and the resulting interaction energy between charged objects is of fundamental importance in scenarios from bio-molecular interactions to energy storage. The conventional wisdom is that the interaction energy decays exponentially with object separation and the decay length is a decreasing function of ion concentration; the interaction is thus negligible in a concentrated electrolyte. Contrary to this conventional wisdom, we have shown by surface fo...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted manuscript

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Publisher copy:
10.1039/C6FD00250A

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Department:
Trinity College
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Department:
Oxford, MPLS, Chemistry, Physical & Theoretical Chem
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Funding agency for:
Perkin, S
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Funding agency for:
Perez-Martinez, C
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Funding agency for:
Perez-Martinez, C
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Grant:
George F. Carrier Fellowship
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Publisher:
Royal Society of Chemistry Publisher's website
Journal:
Faraday Discussions Journal website
Volume:
199
Pages:
239-259
Publication date:
2017-01-05
Acceptance date:
2017-01-27
DOI:
EISSN:
1364-5498
ISSN:
1359-6640
Pubs id:
pubs:677362
URN:
uri:5aae3cc9-a9ae-4cef-a534-a590b04fd461
UUID:
uuid:5aae3cc9-a9ae-4cef-a534-a590b04fd461
Local pid:
pubs:677362

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