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Synthesis of fluorinated alkyl aryl ethers by palladium-catalyzed C–O cross-coupling

Abstract:
Herein, we report a highly effective protocol for the cross-coupling of (hetero)aryl bromides with fluorinated alcohols using the commercially available precatalyst tBuBrettPhos Pd G3 and Cs2CO3 in toluene. This Pd-catalyzed coupling features a short reaction time, excellent functional group tolerance, and compatibility with electron-rich and -poor (hetero)arenes. The method provides access to 18F-labeled trifluoroethyl ethers by cross-coupling with [18F]trifluoroethanol.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/acs.orglett.0c02347

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Organic Chemistry
Role:
Author
ORCID:
0000-0003-1351-1750
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Organic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Organic Chemistry
Role:
Author


Publisher:
American Chemical Society
Journal:
Organic Letters More from this journal
Volume:
22
Issue:
16
Pages:
6573–6577
Publication date:
2020-08-04
Acceptance date:
2020-07-27
DOI:
EISSN:
1523-7052
ISSN:
1523-7060


Language:
English
Keywords:
Pubs id:
1123567
Local pid:
pubs:1123567
Deposit date:
2020-08-05

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